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Optical properties of solids. Branches of physics. This volume 2 introduces lasers and quantum optics, while the main focus is on the structure of molecules and their spectroscopy, as well as on collision physics as the continuum counterpart to bound molecular states.
The emphasis is always on the experiment and its interpretation, while the necessary theory is introduced from this perspective in a compact and occasionally somewhat heuristic manner, easy to follow even for beginners. Country of publication.
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Descriptors DEI. Descriptors DEC. Publication Year Publication Year. Language Language. Reference Number Reference Number. Close Proceed. Export to Mendeley. The existing literature consists of either configuration-averaged distorted-wave or semi-empirical data. Level-resolved rate coefficients are necessary for accurate modeling and diagnostics in plasmas containing argon. We present our level-resolved results and c ompare with existing datasets, finding significant differences. Calculations of the sensitivities of rotational and rovibrational transitions of isotopic lithium hydride in the electronic ground state to a variation of the proton-to-electron mass ratio constant are presented.
A highly enhanced sensitivity coefficient is observed for the splitting of near resonant transitions arising from a cancellation between rotational intervals and frequency shifts associated respectively to the isotope effect, to the anharmonicity and to the rotation-vibration interaction. It ranges from 73 From this experimental information we derived the L 1 , L 2 and L 3 subshell ionization cross sections with a novel analysis procedure that is based on an overdetermined system of equations and achieve the estimates by the least-squares method.
Our experimental results are in reasonable accord with most of the measurements carried out by other authors, and they agree with the predictions of the semi-relativistic distorted-wave Born approximation. We report new experimental and theoretical triple differential cross sections for the electron impact ionization of the three valence states of ammonia in an intermediate energy regime. Measurements are performed in an asymmetric coplanar geometry under kinematics which have been unexplored to date.
The data are compared to predictions from the first order approaches and BBK model. The experimental cross sections exhibit a very large recoil scattering, which is not predicted by the theory. We formulate a nonrelativistic quantum theory for the nonresonant inelastic scattering process of an x-ray photon by a free linear molecule outside of the impulse approximation framework. We find a strong orientation effect dependent on changes in the schemes of the proposed experiments.
Calculations of the absolute values and forms for the double differential scattering cross sections are carried out for the HF molecule and have a predictive character. The presented theory is of a general nature, and its applicability to a particular linear molecule is constrained only by the demand of correctness of nonrelativistic methods for constructing molecular scattering orbitals.
We have performed a kinematically complete experiment on ionization of H 2 by 75 keV proton impact leading to electrons with a speed equal to the projectile speed. By comparing cross sections measured with a coherent and an incoherent projectile beam we were able to perform a detailed analysis of interference effects. We found that the interference structure is significantly more damped than for a smaller electron energy studied previously. This damping is further increased if kinematic conditions are selected which favor a strong role of the post-collisional interaction between the scattered projectile and the electron ejected to the continuum by a preceding primary interaction with the projectile.
Wavepacket propagation calculations are reported for the interaction of a Rydberg hydrogen atom with Cu and Cu surfaces represented by a Chulkov potential , in comparison with a Jellium surface. Both copper surfaces have a projected band gap at the surface in the energy range degenerate with some or all of the Rydberg energies.
The charge transfer of the Rydberg electron to the surface is found to be enhanced for n values at which there is a near-degeneracy between the Rydberg energy level and an image state or a surface state of the surface. The enhancement is facilitated by the strong overlap of the surface image-state orbital lying outside the surface and the orbital of the incoming Rydberg atom. These calculations point to the possibility of using Rydberg-surface collisions as a probe of surface electronic structure.
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Positronium Ps formation processes from helium ions by positron impact are studied using the two-channel two-center eikonal final state—continuum initial distorted wave method. It is found that the present results agree reasonably well with the close-coupling calculations, while other predictions, such as the Coulomb—Born approximation, the optical potential method, and the recent classical trajectory Monte Carlo method Naginey Phys. A 89 , , are all much higher in the entire energy region. The maximum positions of the Ps n formation cross sections in our present work are in good agreement with the wave vector matching model of Charlton J.
B: At. Finally, we discuss the scaling law of the Ps n formation cross sections with respect to the principal quantum number n of the Ps atom. We study the formation and dynamics of shock waves initiated by a repulsive potential in a superfluid unitary Fermi gas by using the order-parameter equation. In the theoretical framework, the regularization process of shock waves mediated by the quantum pressure term is purely dispersive. Our results show good agreement with the experiment of Joseph et al Phys. We reveal that the boxlike-shaped density peak observed in the experiment consists of many vortex rings due to the transverse instability of the dispersive shock wave.
In addition, we study the transition from a sound wave to subsonic shock waves as the strength of the repulsive potential increases and show a strong qualitative change in the propagation speed of the wavefronts. For a relatively small strength of the repulsive potential, the propagation speed decreases below the sound speed with the increase of the strength as a scaling behavior.
For a large strength where the shock waves are formed by colliding two spatially separated clouds, the speed is still smaller than the sound speed, but remains almost unchanged as the strength increases, which can be interpreted as the same expansion speed of the proliferation of the vortex rings originated from the transverse instability.
We have investigated the heteronuclear collision trap loss rates for each isotope due to the presence of cold atoms of other isotope using the TIMOT loading curves. The two body heteronuclear loss rate coefficient i. The dependence of heteronuclear cold collision loss rate on cooling laser beams intensity has also been studied and compared with homonuclear cold collision loss rate.